Sugarland
In 2003, Nettles teamed up with Kristen Hall and Kristian Bush to form Sugarland. Regarding the trio's collaboration, she said:
"We really wanted to get out of where we had all been as artists and move beyond that to something bigger. Consequently all the songs reflect that; 'Fly Away,' 'Baby Girl,' all of those songs - you speak to the human condition and write what you know in your life."
Sugarland was nominated for a Grammy award in the Best New Artist category in 2006. Although they did not win the award, Nettles and Bush performed for the awards show and Nettles presented both a Lifetime Achievement Award to Merle Haggard and the award for Best Country Group.
A duet performance with rock band Bon Jovi, "Who Says You Can't Go Home", reached No. 7 on the Bubbling Under Hot 100 chart and No. 1 on the Billboard Hot Country Singles chart. The video for the song won a CMT Music Award in 2006 for Collaborative Video Of The Year. In February 2007, Nettles and Bon Jovi won a Grammy for Best Country Vocal Collaboration. In 2006, Kristen Hall left the group and Nettles and Bush continued on as a duo releasing Enjoy the Ride in November 2006. Their third album, titled Love on the Inside, was released on July 22, 2008.
In an interview on Fox News with Martha MacCullum, Nettles expressed interest in appearing in a Broadway play, stating in particular that she would like to play the role of Elphaba in Wicked.
In early December 2008, Sugarland received three Grammy Award nominations and performed on the 51st Annual Grammy Awards show on February 8, 2009. They won awards for Best Country Song and Best Country Performance by a Duo or Group.
On Sunday, January 18, 2009, Nettles performed at the We Are One: The Obama Inaugural Celebration at the Lincoln Memorial, singing James Taylor's "Shower the People" with James Taylor and John Legend.
On February 11, 2009, Sugarland received two nominations from the Academy of Country Music for Top Vocal Duo and Vocal Event of the Year for "Life in a Northern Town". During the broadcast of the April 5, 2009 awards show, Sugarland was presented with the Vocal Duo of the Year award, ending Brooks & Dunn's nine-year run. Nettles also received a Milestone award, presented to her by Reba McEntire.
ABC-TV broadcast the first CMA Country Christmas, hosted by Nettles, on November 29, 2010. Nettles and Sugarland partner Kristian Bush kicked off the evening with their rendition of "Winter Wonderland," backed by the Southern harmonies of Little Big Town. The pair returned to the stage later in the program to perform the hymn "Come, O Come Emmanuel," just before the "Jingle Bell Rock" group grande finale of the 90-minute special.
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